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Updated: Jun 3, 2025

Speciation and Bioavailability Measurements of Environmental Plutonium Using Diffusion in Thin Films
Published on: November 9, 2015
Plutonium Marker for the Great Acceleration by Intensified Human Activities
Xue Zhao1,2, Xiaolin Hou1, Weijian Zhou1,2,3
1Xi'an AMS Center, State Key Laboratory of Loess Science, Shaanxi Key Laboratory of Accelerator Mass Spectrometry Technology and Application, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, P. R. China.
Plutonium-239,240 (Pu) from nuclear tests provides a marker for the Great Acceleration. Its deposition and preservation in lake sediments offer a robust timeline for this significant human-impact period.
Area of Science:
- Environmental Science
- Geochemistry
- Nuclear Science
Background:
- Human activities surged in the mid-20th century, termed the Great Acceleration.
- Nuclear activities are a defining technological process of this era.
- Plutonium-239,240 (Pu) fallout from nuclear weapons tests is a potential chronostratigraphic marker, but its sediment accumulation dynamics are debated.
Purpose of the Study:
- To analyze plutonium-239,240 (Pu) in lake sediment cores to establish a precise timeline for the Great Acceleration.
- To investigate the accumulation dynamics of Pu from atmospheric deposition to sediment preservation in different lake environments.
Main Methods:
- Analysis of three sediment cores from two maar lakes with established chronologies.
- Measurement of plutonium-239,240 (Pu) concentrations within the sediment layers.
Main Results:
- The first significant increase in Pu-239,240 was observed in 1953, corresponding to the first high-yield thermonuclear test.
- Pu-239,240 peaked in 1963, aligning with the period of highest global nuclear testing.
- Pu scavenging and preservation dynamics differed between anoxic (Lake Sihailongwan) and oxic (Lake Huguangyan) lake environments.
Conclusions:
- Pu-239,240 deposition in lake sediments serves as a robust and permanent marker for the Great Acceleration.
- The identified Pu timeline (1953 increase, 1963 peak) accurately reflects major nuclear events and human impact.
- Lake sediments, particularly in anoxic environments, provide excellent archives for preserving this nuclear chronostratigraphic marker.
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