Related Experiment Video
Updated: May 30, 2025

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Modulation of electron correlation dynamics in atomic non-sequential double ionization by counter-rotating two-color
Abstract:
We investigate the ultrafast electron correlation effects during non-sequential double ionization (NSDI) of argon subjected to a combined femtosecond field composed of counter-rotating two-color circularly polarized (TCCP) pulse laser using a 3D classical ensemble model (CEM). Our simulation results reveal that manipulation of the carrier-envelope phase (CEP) of the external driving field modulates the dynamical behavior of the two electrons, resulting in a notable sensitivity of their momentum distribution to the relative phase of two components of the counter-rotating TCCP field. Through inversion analysis, we uncover the capability to direct electrons toward a single direction, thereby facilitating focused ion-electron collisions on the attosecond timescale. Furthermore, we observe that adjusting the CEP exerts a substantial influence on the NSDI ionization process, modifying the relative contributions of the recollision-induced ionization (RII) mechanism and recollision excitation with subsequent ionization (RESI) mechanism.
Related Concept Videos
Molecular Orbital Theory I
Deactivation Processes: Jablonski Diagram
π Electron Effects on Chemical Shift: Overview
Crystal Field Theory - Octahedral Complexes
To explain the observed behavior of transition metal complexes (such as colors), a model involving electrostatic interactions between the electrons from the ligands and the electrons in the unhybridized d orbitals of the central metal atom has been developed. This electrostatic model is crystal field theory (CFT). It helps to understand, interpret, and predict the colors, magnetic behavior, and some structures of coordination compounds of transition metals.
CFT focuses on...
Molecular Orbital Theory II
Double Resonance Techniques: Overview
Spin decoupling is usually achieved by...

