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Combining Microfluidics and Microrheology to Determine Rheological Properties of Soft Matter during Repeated Phase Transitions
Published on: April 19, 2018
Steady inhomogeneous shear flows as mechanical phase transitions
1University of Stuttgart, Institute for Theoretical Physics IV, Heisenbergstr. 3, 70569 Stuttgart, Germany.
This study introduces a mechanical framework to understand inhomogeneous fluid flows and shear banding. It provides a new theoretical approach for systems far from thermal equilibrium, applicable to complex fluids and solid-melt coexistence.
Area of Science:
- Non-equilibrium statistical mechanics
- Fluid dynamics
- Materials science
Background:
- Inhomogeneous flows and shear banding lack comprehensive theoretical understanding.
- Existing frameworks do not adequately address systems far from thermal equilibrium.
- A need exists for a mechanical equilibrium approach.
Purpose of the Study:
- To develop a theoretical framework for understanding inhomogeneous flows and shear banding.
- To apply a mechanical equilibrium concept to non-equilibrium systems.
- To illustrate the framework with applications in complex fluids and solid-melt systems.
Main Methods:
- Revisiting models of fluids in stationary states obeying mechanical equilibrium.
- Utilizing a nonlocal constitutive relation.
- Applying the concept of a "mechanical phase transition" and mapping to a dynamical system via an integrating factor.
Main Results:
- A novel mechanical framework for inhomogeneous systems away from thermal equilibrium.
- Successful application to shear banding in complex fluids.
- Demonstration of solid-melt coexistence using the proposed framework.
Conclusions:
- The developed mechanical framework offers a new route to describe inhomogeneous systems.
- This approach provides insights into shear banding and phase coexistence phenomena.
- The study contributes to a deeper understanding of non-equilibrium fluid mechanics.
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