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Updated: May 23, 2025

Spectral and Angle-Resolved Magneto-Optical Characterization of Photonic Nanostructures
Published on: November 21, 2019
Infrared Magnetopolaritons in MoTe_{2} Monolayers and Bilayers
Bo Han1, Jamie M Fitzgerald2, Lukas Lackner1
1Carl von Ossietzky Universität Oldenburg, Institut für Physik, Fakultät V, 26129 Oldenburg, Germany.
Abstract:
MoTe_{2} monolayers and bilayers are unique within the family of van der Waals materials since they pave the way toward atomically thin infrared light-matter quantum interfaces, potentially reaching the important telecommunication windows. Here, we report emergent exciton polaritons based on MoTe_{2} monolayers and bilayers in a low-temperature open microcavity in a joint experiment-theory study. Our experiments clearly evidence both the enhanced oscillator strength and enhanced luminescence of MoTe_{2} bilayers, signified by a 38% increase of the Rabi splitting and a strongly enhanced relaxation of polaritons to low-energy states. The latter is distinct from polaritons in MoTe_{2} monolayers, which feature a bottlenecklike relaxation inhibition. Both the polaritonic spin valley locking in monolayers and the spin-layer locking in bilayers are revealed via the Zeeman effect, which we map and control via the light-matter composition of our polaritonic resonances.
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