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Cooper-pair density modulation state in an iron-based superconductor.

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Researchers discovered a new superconducting state called pair density modulation (PDM) in iron-based superconductors. This state preserves lattice translation, unlike previous density-wave orders, and offers new insights into complex electronic systems.

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Area of Science:

  • Condensed Matter Physics
  • Materials Science
  • Quantum Materials

Background:

  • Superconducting states can break crystal space-group symmetries, leading to density-wave orders with long wavelengths.
  • A distinct type of modulation, pair density modulation (PDM), preserving lattice translation by breaking intra-unit-cell symmetries, has been theoretically proposed but experimentally elusive.

Purpose of the Study:

  • To report the first experimental observation of a pair density modulation (PDM) state.
  • To investigate the characteristics and origin of PDM in iron-based superconductors.

Main Methods:

  • Utilized scanning tunnelling microscopy (STM) to probe the electronic properties of exfoliated thin flakes of FeTe$_{0.55}$Se$_{0.45}$.
  • Performed model calculations to support experimental findings and elucidate the underlying physics.

Main Results:

  • Observed robust superconducting gap modulation with a wavelength matching the lattice periodicity in FeTe$_{0.55}$Se$_{0.45}$ thin flakes.
  • The amplitude of the gap modulation exceeded 30% of the average superconducting gap.
  • The PDM state was found to originate from differences in superconducting gaps between iron sublattices, coupled with nematic distortion in thin flakes.

Conclusions:

  • Established the first experimental evidence for pair density modulation (PDM) in a superconducting material.
  • Demonstrated that PDM arises from sublattice symmetry breaking and nematicity, distinct from density-wave orders.
  • Opened new avenues for exploring intertwined orders in strongly correlated electronic systems and advanced the understanding of iron-based superconductors.