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Updated: May 16, 2025

Compact Quantum Dots for Single-molecule Imaging
Published on: October 9, 2012
Quantum dots enhanced stability of in-situ fabricated perovskite nanocrystals based light-emitting diodes: Electrical
Xulan Xue1, Menglin Li2, Zhenjie Liu1
1Key Lab of Physics and Technology for Advanced Batteries (Ministry of Education), College of Physics, Jilin University, Changchun 130012, China.
Abstract:
With the development in fabricating efficient perovskite light emitting diodes (PeLEDs), improving the operating stability becomes an urgent task. Here we report quantum dot (QD) enhanced stability of PeLEDs by introducing CdSe/ZnS core-shell QDs in toluene anti-solvent during in-situ fabrication of FAPbBr3 perovskite nanocrystals (PNCs) films. In comparison with PNC films with pristine toluene as the anti-solvent, the as-prepared FAPbBr3 PNC films with a QD monolayer on the surface exhibit improved photoluminescence quantum yield, enhanced photostability and better reproducibility. Benefiting from these advantages, the peak luminance and the maximum external quantum efficiency of the PeLED containing QD monolayer are increased from 6807 cd/m2 to 86,670 cd/m2 and 2.4% to 7.1%, respectively. The T 50 lifetime under the initial luminance of 1021 cd/m2 approaches 83 minutes. Based on electrical field simulation and transient electroluminescence measurements, the enhanced stability can be mainly attributed to the electrical field redistribution induced by the QD monolayer. This work demonstrates that the combination of QDs and perovskites provides an effective strategy to address the operational stability of PeLEDs. The insights into electrical field distribution effect will make great impact on stability improvement of other perovskite based devices.
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