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A Decade of Lead Halide Perovskites for Direct-Conversion X-ray and Gamma Detection: Technology Readiness Level and
Kostiantyn Sakhatskyi1,2, Aditya Bhardwaj1,2, Gebhard J Matt1,2
1Laboratory of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, Zürich, CH-8093, Switzerland.
Lead halide perovskites (LHPs) are revolutionizing radiation detection. This review summarizes a decade of advancements in LHP detectors for X-ray and gamma-ray applications, highlighting progress and future challenges.
Area of Science:
- Materials Science
- Physics
- Engineering
Background:
- Lead halide perovskites (LHPs) have emerged as promising materials for radiation detection.
- They offer cost-effective and robust alternatives to traditional semiconductor detectors.
- Their unique properties make them suitable for high-energy radiation detection.
Purpose of the Study:
- To review the advancements in lead halide perovskite radiation detectors over the past decade.
- To highlight material, structural, and functional progress in the field.
- To identify challenges hindering the widespread adoption of LHP detectors.
Main Methods:
- Comprehensive literature review of perovskite radiation detector research.
- Analysis of material properties, synthesis techniques, and device architectures.
- Discussion of stability, efficiency, scalability, and imaging applications.
Main Results:
- Significant progress in material synthesis and processing has improved detector stability, efficiency, and scalability.
- Evolution of device architectures from single-channel to multi-pixel arrays for imaging.
- Identification of key properties like high atomic number, charge carrier mobility, and resistivity.
Conclusions:
- LHP radiation detectors have shown remarkable progress in their first decade.
- Further research is needed to overcome remaining challenges for technological advancement.
- The field shows strong potential for future development in X-ray and gamma-ray detection.
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