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Constructing VN-V2O3 Heterogeneous Interface to Improve Wide Temperature Zinc Storage Performance.

Fuyu Xiao1, Hui Lin1, Ziyan Yuan1

  • 1Engineering Research Center of Polymer Green Recycling of Ministry of Education, Fujian Key Laboratory of Pollution Control & Resource Reuse, College of Environmental and Resources, Fujian Normal University, Fuzhou, Fujian, 350007, China.

Small (Weinheim an Der Bergstrasse, Germany)
|May 24, 2025
PubMed
Summary
This summary is machine-generated.

This study introduces a novel porous vanadium nitride-vanadium oxide (VN-V2O3) heterostructure for high-performance aqueous zinc-ion batteries (ZIBs). The material offers excellent capacity, long cycle life, and stable operation across a wide temperature range.

Keywords:
heterogeneous interfacevanadium‐based materialwide temperature performancezinc‐ion battery

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Vanadium-based materials offer high capacity for zinc storage but suffer from dissolution and poor low-temperature performance.
  • Challenges in vanadium-based cathodes include capacity decay and slow ion transport, limiting their practical application in aqueous zinc-ion batteries (ZIBs).

Purpose of the Study:

  • To develop a novel vanadium nitride-vanadium oxide (VN-V2O3) heterostructure to overcome the limitations of vanadium-based cathode materials.
  • To enhance zinc ion (Zn2+) storage, ion diffusion, and electrochemical performance in aqueous ZIBs.

Main Methods:

  • Fabrication of a porous VN-V2O3 heterostructure using a solvothermal and pyrolysis method.
  • Electrochemical testing of the VN-V2O3 electrode in an aqueous zinc-ion battery system with a gel electrolyte.

Main Results:

  • The VN-V2O3 heterostructure exhibits a high reversible capacity of 335 mAh g-1.
  • Achieved ultra-long cycling stability with 6000 cycles at 10 A g-1.
  • Demonstrated excellent zinc storage performance over a wide temperature range (-35 to 60 °C).

Conclusions:

  • The developed VN-V2O3 heterostructure provides a feasible strategy for achieving long cycle stability and wide temperature adaptability in cathode materials for aqueous ZIBs.
  • This work offers a new reference for constructing vanadium-based heterostructures for advanced energy storage applications.