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Validation of simulated training sets using a convolutional neural network for isotope identification in urban
Luke Lee-Brewin1, Ryan Holden1, Caroline Shenton-Taylor1
1Physics, University of Surrey, Guildford, Surrey, United Kingdom.
Plos One
|June 9, 2025
Summary
This study validates a novel method for generating simulated gamma spectra, crucial for training neural networks in real-time isotope identification for law enforcement. The approach successfully identified isotopes in urban environments, achieving high prediction accuracy.
Area of Science:
- Nuclear physics and instrumentation
- Artificial intelligence and machine learning
- Public safety and security
Background:
- Real-time isotope identification in urban settings is vital for law enforcement threat assessment.
- Challenges exist in creating representative training datasets for neural networks due to variable urban conditions.
- Existing methods struggle with the wide range of isotopes, activities, and shielding encountered.
Purpose of the Study:
- To validate a method for generating realistic gamma spectra datasets without radioactive sources.
- To train and test a convolutional neural network (CNN) for isotope identification using simulated and real-world data.
- To assess the feasibility of using generated spectra for accurate isotope detection in uncontrolled environments.
Main Methods:
- Generated synthetic gamma spectra by combining simulated isotope signatures with background radiation from the SIGMA dataset.
- Utilized k-means clustering to extract a labeled dataset of 12,748 spectra from the SIGMA dataset.
- Trained a CNN classifier on the combined simulated and real-world spectral data.
Main Results:
- The CNN model achieved high prediction accuracy, with the lowest class accuracy at 96% for simulated data and 89.8% for real SIGMA dataset spectra.
- The method successfully identified isotopes within real-world gamma spectra from the SIGMA dataset.
- Validation confirmed the effectiveness of the simulated data generation technique.
Conclusions:
- The validated method for generating gamma spectra is effective for training isotope identification models.
- This approach significantly aids in developing robust AI tools for real-time threat detection in urban environments.
- Future work can expand the isotopic library and model complexity for enhanced security applications.

