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Acoustic Manipulation of Deterministic Quantum Emitters in WSe2
Seyed Sepehr Mohajerani1,2, Adnane Noual1,3, Yichen Ma1,2
1Department of Physics, Stevens Institute of Technology, Hoboken, New Jersey 07030, United States.
ACS Nano
|July 9, 2025
Summary
Surface acoustic waves (SAWs) enable high-speed control of quantum emitters in 2D materials. This study demonstrates acoustic manipulation of strain-induced quantum emitters in WSe2 for fast optical modulation.
Area of Science:
- Quantum physics
- Materials science
- Nanotechnology
Background:
- Surface acoustic waves (SAWs) are used to control excitonic states in 2D materials.
- High-speed manipulation of site-controlled quantum emitters (QEs) in 2D materials using SAWs is underexplored.
Purpose of the Study:
- To demonstrate acoustic manipulation of deterministic, strain-induced QEs in monolayer WSe2.
- To achieve high-speed optical modulation of QEs using SAWs.
Main Methods:
- Interfacing monolayer WSe2 with SAWs on a lithium niobate substrate.
- Using gold nanocube stressors to engineer local strain for deterministic QEs.
- Exciting QEs with SAWs and measuring energy shifts and modulation speeds.
Main Results:
- Deterministic QEs in WSe2 exhibited energy shifts up to 0.58 meV with an 8 MHz tuning bandwidth.
- Achieved half-GHz optical modulation speed for QEs located 210 nm above the substrate.
- Revealed a nonlinear response regime of the SAW-driven nanocube stressor.
Conclusions:
- Acoustic manipulation provides a robust and scalable approach for fast, dynamic tuning of single photons.
- The developed method offers suppressed spectral diffusion and potential for nanoscale quantum sensors.
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