Efficient CO2 conversion enabled by well-dispersed Co nanoparticles on N-doped hollow-structured carbon supports
1The Key Laboratory of Functional Molecular Solids Ministry of Education, College of Chemistry and Materials Science, Anhui Normal University, Wuhu 214001, P. R. China. ruirui58@ahnu.edu.cn.
Abstract
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An exceptional catalyst featuring uniformly dispersed cobalt nanoparticles on a hollow structure was fabricated. Both experimental and theoretical results demonstrate that the N-doped support modulates the electron density of the active sites. At the same time, the hollow architecture facilitates substrate enrichment, collectively enhancing CO2 fixation and leading to superb catalytic activity and excellent cycling stability.


