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Multi-Stimulus Soft Actuators from Aerosol Jet Printed MXene-Cellulose Composite
Brian Cole1, Yilin Zhao1, Anna Bethke2
1Department of Electrical & Computer Engineering, Duke University, Durham, North Carolina 27708, United States.
Nano Letters
|October 20, 2025
Summary
Researchers developed a new method for creating soft robotic actuators using aerosol jet printing of transition metal carbide (TMC, MXene) and cellulose nanofiber (CNF) composites. This scalable technique enables customizable, multi-stimulus responsive microrobots.
Area of Science:
- Materials Science
- Robotics Engineering
- Nanotechnology
Background:
- Advancements in flexible, stretchable, and conformal microrobotics require improved fabrication methods.
- Current methods face limitations in actuator feature scalability and design versatility.
Purpose of the Study:
- To demonstrate additive manufacturing of soft multi-stimulus thermomechanical actuators.
- To utilize a composite of transition metal carbide (TMC, MXene) and cellulose nanofiber (CNF) nanomaterials.
- To achieve scalable and customizable actuation using aerosol jet printing (AJP).
Main Methods:
- Aerosol jet printing (AJP) of aqueous MXene-CNF films onto polycarbonate (PC) membranes.
- Tuning electrothermal and photothermal properties for wired and/or wireless operation.
- Fabricating devices with dimensions as small as 5 mm² and 2.5 mm².
Main Results:
- Achieved full reversibility with heating below 120 °C.
- Demonstrated sharp curvatures of 0.92 cm⁻¹ and 0.87 cm⁻¹ for printed devices.
- Realized complex, directional, and reversible actuation modes by selective printing on both sides of the substrate.
Conclusions:
- AJP-fabricated MXene-CNF systems show significant promise for soft robotics applications.
- The developed method offers enhanced scalability and design versatility for microrobotic actuators.
- The multi-stimulus responsive actuators are suitable for various customizable robotic designs.

