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Reassessing Electrolyte Design for Non-Aqueous Magnesium Batteries: Atomistic Structures and Performance

Hao Xu1,2, Xiaoqian He1, Yue Li3

  • 1National Engineering Research Center of Light Alloy Net Forming & Center of Hydrogen Science, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai, 200240, China.

Advanced Materials (Deerfield Beach, Fla.)
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Summary
This summary is machine-generated.

Developing advanced electrolytes is key for non-aqueous magnesium (Mg) batteries. This review analyzes chlorine-containing and chlorine-free options, highlighting challenges and future directions for Mg battery performance.

Keywords:
atomistic structureschlorine‐containing electrolyteschlorine‐free electrolyteselectrolyte designmagnesium batteries

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Non-aqueous magnesium (Mg) batteries offer high Mg abundance and safety, positioning them as a promising energy storage technology.
  • The practical application of Mg batteries is significantly hindered by the lack of efficient non-aqueous electrolytes.
  • Electrolyte development is critical for overcoming current limitations and enabling widespread Mg battery adoption.

Purpose of the Study:

  • To provide a comprehensive review of recent advancements in non-aqueous electrolytes for Mg batteries.
  • To analyze the challenges and future directions for both chlorine-containing and chlorine-free electrolyte systems.
  • To evaluate the influence of electrolyte design on Mg stripping/plating processes and electrochemical stability.

Main Methods:

  • Literature review and analysis of existing research on non-aqueous electrolytes for Mg batteries.
  • Comparative evaluation of chlorine-containing and chlorine-free electrolyte systems.
  • Discussion of electrolyte design strategies, atomistic structures, and performance optimization.

Main Results:

  • Chlorine-containing electrolytes show high ionic conductivity and reversibility but face issues with corrosion and limited electrochemical stability.
  • Chlorine-free electrolytes present an eco-friendly alternative but often exhibit lower ionic conductivity and poor compatibility with Mg metal anodes.
  • Both electrolyte types present distinct advantages and disadvantages impacting Mg battery performance.

Conclusions:

  • Electrolyte innovation is pivotal for unlocking the full potential of non-aqueous Mg batteries.
  • Addressing challenges in Mg anode compatibility and electrochemical stability is crucial for both electrolyte types.
  • Further research into advanced electrolyte design methodologies is essential for sustainable and high-performance energy storage solutions.