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Encapsulation of CdSe QDs into micellar microreactors for highly selective photocatalytic CO2 reduction in aqueous
Wu Xia1,2, Zi-Hao Liao1, Hong-Fei Li1
1Key Laboratory of Materials Chemistry for Energy Conversion and Storage (Huazhong University of Science and Technology) of Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, 430074, P. R. China. wangfengchem@hust.edu.cn.
None:
Hydrophobic ligand-modification of CdSe QDs allows facile encapsulation of the QDs into SDS micelles, creating a hydrophobic, CO2-enriched microreactor for QDs enabling efficient, highly selective CO2-to-CO photoconversion of 2.47 mmol g-1 and up to 91.5% selectivity, in aqueous solution, outperforming pristine MPA-CdSe and MUA-CdSe.
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