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Area of Science:

  • Optics and Photonics
  • Materials Science
  • Nanotechnology

Background:

  • Controlling polarization, wavefront, and directionality of lasing emission is crucial for optical technologies.
  • Independent tunability of these characteristics in a single cavity remains a significant challenge.
  • Dielectric metasurfaces offer wavefront control but often lack high-quality cavity modes for lasing.

Purpose of the Study:

  • To demonstrate plasmonic cavities capable of supporting phase-gradient lattice resonances.
  • To achieve strong coupling between excitons and chiral cavity modes for tunable lasing.
  • To enable simultaneous control over spin and orbital angular momentum in laser beams.

Main Methods:

  • Utilizing plasmonic cavities to support phase-gradient lattice resonances.
  • Employing Cadmium Selenide (CdSe) nanoplatelets for exciton coupling.
  • Engineering localized plasmons to manipulate phase singularities and geometric phase.

Main Results:

  • Achieved unity circular polarization at engineered Fourier space positions.
  • Demonstrated strong exciton-cavity coupling, yielding photoluminescence with near-unity chirality.
  • Obtained low-threshold, simultaneous lasing from multiple beams with tunable angles.

Conclusions:

  • Plasmonic cavities can support engineered phase-gradient lattice resonances for lasing.
  • Strong coupling enables generation of chiral light with tunable properties.
  • This work highlights the potential of localized plasmons for precise control of light angular momentum.