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MoO2‑Doped Li7P3S11 for High-Performance All-Solid-State Lithium Batteries.

Ziheng Zhao1, Yuan Hua1, Peng Hang2

  • 1School of Chemical and Environmental Engineering, Wuhan Institute of Technology, Wuhan 430205, P. R. China.

ACS Omega
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Researchers enhanced sulfide solid electrolytes for all-solid-state lithium batteries (ASSLBs) by codoping with MoO2. This improves ionic conductivity and air stability, enabling stable battery cycling and higher capacity retention.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Solid-State Batteries

Background:

  • Sulfide electrolytes are promising for all-solid-state lithium batteries (ASSLBs) due to their amorphous structure and softness.
  • Key challenges include low ionic conductivity, poor lithium compatibility, and limited air stability.

Purpose of the Study:

  • To develop a novel codoping strategy for glassy sulfide electrolytes.
  • To enhance ionic conductivity, lithium compatibility, and air stability of Li7P3S11-based electrolytes.

Main Methods:

  • Incorporation of MoO2 into Li7P3S11 via a codoping strategy.
  • Fabrication and electrochemical testing of symmetric and full cells using the optimized electrolyte.

Main Results:

  • Achieved an ionic conductivity of 2.57 mS/cm at room temperature.
  • Demonstrated enhanced air stability and suppressed H2S generation.
  • Symmetric cells showed stable cycling over 400 hours at 0.7 mA cm-2.
  • Full cells exhibited 122.47 mAh·g-1 initial capacity and 77.31% retention after 100 cycles.

Conclusions:

  • Codoping with MoO2 effectively improves ionic conductivity and air stability of sulfide electrolytes.
  • The developed electrolyte shows potential for dendrite suppression and enhanced performance in ASSLBs.