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Polarization-Resolved Terahertz Near-Field Nanoscopy of Graphene
Ran Wang1,2,3,4, Zhuocheng Zhang1,2,3,4, Xiaoqiuyan Zhang1,2,3,4
1Terahertz Research Center, School of Electronic Science and Engineering, University of Electronic Science and Technology of China, Chengdu 611731, China.
None:
Scattering-type scanning near-field optical microscopy (s-SNOM) provides access to nanoscale optical responses beyond the diffraction limit. However, at low terahertz (THz) frequencies, quasi-electrostatic models predict that highly conductive graphene behaves as a near-total reflector to large in-plane-momentum (q) near fields, essentially insensitive to layer number. Here, we probe graphene from monolayer to few-layer using polarization-resolved terahertz near-field nanoscopy with cross-polarized detection. We find that the p-polarized near-field signal rapidly reaches a saturation level, whereas the orthogonal s-polarized channel retains a clear, layer-dependent contrast. Theoretical modeling shows that this contrast arises from the in-plane reflection coefficient (rs), which increases approximately linearly with the conductivity of graphene in the high-q regime. Together, our results clarify how p- and s-polarized fields couple differently to the tip-sample system, establish a physical framework for polarization-dependent terahertz near-field responses, and point to multidimensional nanoscopic detection schemes for anisotropic materials.
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