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Updated: Feb 15, 2026

Hyperspectral Imaging as a Tool to Study Optical Anisotropy in Lanthanide-Based Molecular Single Crystals
Published on: April 14, 2020
Hyperspectral imaging of downconverted photons in angle phase-matched nonlinear crystals
Abstract:
Spontaneous Parametric Downconversion (SPDC) is key to generating broadband spectrally entangled photons for quantum optical spectroscopy. Here, we use a common-path birefringent interferometer to experimentally map the spatial-spectral distribution of SPDC in Type I and II β-barium borate crystals using hyperspectral k-space imaging. Under broadband pulsed pumping, we observe strong spatial variations in the spectra, with distinct features for each phase-matching type. Simulations based on biphoton amplitudes and phase-matching conditions qualitatively match our results. This spatial-spectral mapping enables control over biphoton entanglement entropy, paving the way for optimized quantum-light sources for material spectroscopy.
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