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Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy
Published on: January 20, 2023
Perspective on Material Design and Interface Engineering toward Low-Stack-Pressure All-Solid-State Lithium Batteries
Shenghan Gao1,2, Wen-Peng Wang1,2, Li-Jun Wan1,2
1CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory For Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing, P. R. China.
All-solid-state lithium batteries (ASSLBs) need high pressure for good performance. This review explores solutions for low-pressure ASSLBs, focusing on materials and interfaces for better energy storage.
Area of Science:
- Materials Science
- Electrochemistry
- Energy Storage
Background:
- All-solid-state lithium batteries (ASSLBs) offer high energy density and safety.
- Poor solid-solid interfacial contact limits ASSLB cyclability and requires high stack pressure.
- Current limitations hinder the commercialization of ASSLBs.
Purpose of the Study:
- To provide a fundamental understanding of stack pressure's role in ASSLBs.
- To analyze challenges in achieving optimal performance under low-stack-pressure conditions.
- To summarize recent advances in reducing high-stack-pressure demands.
Main Methods:
- Review of existing literature on ASSLB stack pressure.
- Analysis of material design (solid electrolyte/active electrode) for low-pressure operation.
- Examination of interface engineering strategies.
Main Results:
- High stack pressure is often necessary due to interfacial resistance.
- Material-centered solutions and interface engineering are key to reducing pressure requirements.
- Progress has been made in designing components for low-pressure ASSLBs.
Conclusions:
- Achieving low-stack-pressure ASSLBs is crucial for commercialization.
- Future breakthroughs require continued focus on material design and interface engineering.
- Material-centered solutions hold promise for advancing battery technology.
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