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Updated: May 13, 2026

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Fabrication of Gate-tunable Graphene Devices for Scanning Tunneling Microscopy Studies with Coulomb Impurities
Published on: July 24, 2015
Precisely Controllable Generation and Characterization of Graphene Nanogaps
Chong Liu1, Menglan Li1,2, Fenfa Yao3
1Key Laboratory for the Physics and Chemistry of Nanodevices, School of Electronics, Peking University, Beijing 100871, China.
Nano Letters
|May 12, 2026
Summary
Researchers developed a deterministic method for fabricating single-layer graphene nanogaps. This technique precisely controls electric breakdown, enabling high-yield production of sub-3 nm gaps for single-molecule devices.
Area of Science:
- Materials Science
- Nanotechnology
- Electrical Engineering
Background:
- Sub-3 nm nanogaps are critical for single-molecule electronic devices.
- Existing fabrication methods are stochastic, leading to inconsistent nanogap sizes and resistance distributions.
Purpose of the Study:
- To present a deterministic method for precise single-layer graphene nanogap fabrication.
- To overcome the limitations of stochastic fabrication techniques for nanogap devices.
Main Methods:
- Controlled electric breakdown of single-layer graphene.
- Utilizing autoranging source-measure hardware with distinct control logics before and after breakdown.
- Direct visualization of nanogaps using transmission electron microscopy.
Main Results:
- Achieved deterministic generation of single-layer graphene nanogaps with sub-3 nm separations.
- Approximately 80% of fabricated devices exhibited nanogap resistance within the same order of magnitude.
- Demonstrated tunability of nanogap resistance via the termination parameter.
Conclusions:
- Established a robust and controllable approach for fabricating single-layer graphene nanogaps.
- This method facilitates high-yield production of single-molecule junctions and solid-state devices.
- Paves the way for advanced nanoscale electronic applications.

