Fast-Recovery Epitaxial NbN Superconducting Nanowire Single-Photon Detectors with Saturated Efficiency at 1550 nm in...

Achieving both high internal efficiency and fast reset times at elevated temperatures remains challenging due to limited understanding of how film properties govern superconducting nanowire single-photon detector (SNSPD) performance. We demonstrate that epitaxial NbN films on sapphire enable simultaneous high efficiency and rapid response. We fabricate and characterize SNSPDs based on these films deposited via DC magnetron sputtering on c-cut sapphire. High-quality epitaxial growth preserves a low electron diffusion coefficient and promotes strong electron-phonon coupling, yielding a high critical temperature and efficient hotspot formation in the dirty limit. X-ray diffraction and transmission electron microscopy confirm epitaxial alignment and lattice order. Nanowires of 20 nm width exhibit saturated internal efficiency at 1550 nm wavelength and short reset times at 4.2 K, enabled by lattice matching and high thermal conductance of the sapphire interface. Ab initio modeling reproduces photon count rates, linking device performance quantitatively to film properties such as diffusivity and electron-phonon coupling.