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Updated: May 21, 2026

Screening of Coatings for an All-Solid-State Battery Using In Situ Transmission Electron Microscopy

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Published on: January 20, 2023

Decoupling Chemo-Mechanical Degradation for Scalable Silicon-Based Solid-State Batteries.

Yujing Su¹, Yingdong Chen¹, Lei Zhao²

¹School of Chemistry and Chemical Engineering, Nanjing University of Science and Technology, Nanjing, China.

Advanced Materials (Deerfield Beach, Fla.)

|May 20, 2026

Summary

This summary is machine-generated.

Silicon-based solid-state batteries offer higher energy density but face degradation. This review explores failure mechanisms and stabilization strategies for practical Si-SSB development.

Keywords:

chemo‐mechanical degradation interface engineering silicon anode solid electrolytes

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Area of Science:

Materials Science
Electrochemistry
Mechanical Engineering

Background:

Silicon-based solid-state batteries (Si-SSBs) are promising for next-generation energy storage.
Their advancement is hindered by chemo-mechanical degradation at the silicon anode-solid electrolyte interface.

Purpose of the Study:

To systematically review Si-SSB failure mechanisms.
To evaluate strategies for interfacial stabilization and mechanical reinforcement.
To discuss scalability and manufacturing considerations.

Main Methods:

Operando characterization techniques to study failure mechanisms.
Analysis of interfacial stabilization strategies including viscoelastic buffers, surface modification, and composite design.
Multiscale modeling to understand stress-electrochemical coupling.

Main Results:

Detailed understanding of chemo-mechanical degradation pathways at the atomic and macroscopic levels.
Evaluation of various strategies to enhance interfacial stability and mechanical properties.
Identification of key factors for harmonizing ionic conductivity and mechanical compliance.

Conclusions:

Interfacial engineering is crucial for overcoming Si-SSB degradation.
Integrated material design and multiscale modeling are essential for performance optimization.
Addressing scalability and manufacturing challenges is vital for commercialization.