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Updated: Jun 12, 2026

Hyperspectral Imaging as a Tool to Study Optical Anisotropy in Lanthanide-Based Molecular Single Crystals
Published on: April 14, 2020
Hyperspectral Imaging of Dipole-Ladder-Mediated Exciton Drift in Moiré Superlattices
Xiao-Ze Li1, Boyi Xu2,3,4, Ying Jiang2,3,4
1State Key Laboratory of Precision Measurement Technology and Instruments, Department of Precision Instrument, Tsinghua University, Beijing 100084, China.
Abstract:
Moiré superlattices have emerged as a highly tunable platform for exploring correlated bosonic states, such as the recently discovered dipole ladder arising from strong on-site exciton-exciton interactions. Although spectroscopic signatures of these dipole ladders are established, their influence on exciton transport has remained unknown. Here, we employ hyperspectral transient photoluminescence microscopy to directly visualize exciton dynamics in a WS2/WSe2 moiré superlattice and demonstrate that dipole ladder mediates highly efficient exciton drift. At high excitation densities, the formation of a transient dipolar ladder generates a steep internal potential gradient. This gradient triggers a transition from localized, diffusion-limited transport (with a diffusion coefficient of D ≈ 0.01 cm2 s-1) to rapid, drift-dominated flow, yielding an equivalent diffusion coefficient of 0.75 cm2 s-1. These results establish dipole ladders as an interaction-driven mechanism for controlling exciton flow in moiré superlattices.
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