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Updated: Jun 20, 2026

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Infrared Degenerate Four-wave Mixing with Upconversion Detection for Quantitative Gas Sensing
Published on: March 22, 2019
High-Sensitivity Near-Infrared Upconversion Detector Using Hybrid Plasmonic-Photonic Structure
Jianqing Cai1, Yunheng Wang1, Chuheng Fu2
1School of Microelectronics, Southern University of Science and Technology, Shenzhen 518055, China.
ACS Applied Materials & Interfaces
|June 18, 2026
Summary
This study introduces a novel near-infrared (NIR) upconversion detector using UCNPs-PDMS microarrays with plasmonic and photonic elements. The enhanced detector significantly improves NIR imaging performance and detectivity for quantitative sensing applications.
Area of Science:
- Materials Science
- Nanotechnology
- Optical Engineering
Background:
- Near-infrared (NIR) upconversion detectors enable direct imaging by converting NIR light to visible emission, recordable by standard cameras.
- Current detectors face limitations due to weak NIR absorption and nonlinear excitation dynamics, reducing conversion efficiency and device detectivity.
Purpose of the Study:
- To develop a camera-readable NIR upconversion detector with enhanced performance.
- To overcome the limitations of traditional lanthanide-doped upconversion detectors.
Main Methods:
- Integration of a UCNPs-PDMS microarray with cascaded plasmonic (Au nanorods) and photonic (microlens array) field-modulation elements.
- Utilized nanoscale near-field amplification and light concentration to boost upconversion luminescence.
Main Results:
- Achieved over 8-fold enhancement in raw upconversion luminescence.
- Reduced noise-equivalent irradiance (NEI) from 83.98 to 0.674 mW·cm⁻².
- Increased effective optical-readout specific detectivity from 2.17 × 10³ to 2.70 × 10⁵ Jones, a 124.6-fold improvement.
Conclusions:
- The developed cascaded hybrid architecture significantly enhances NIR upconversion detector performance.
- Demonstrated stable, quantitative optical-readout monitoring for time-lapse drying, validating its sensing capabilities.
- The detector offers a promising solution for advanced NIR imaging and sensing applications.
Keywords:
microlens arraynear-infrared detectionoptical readoutplasmonic enhancementupconversion nanoparticles
