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Low Pressure Vapor-assisted Solution Process for Tunable Band Gap Pinhole-free Methylammonium Lead Halide Perovskite Films
Published on: September 8, 2017
High-performance multijunction perovskite LEDs with reduced interconnection loss
Feiyun Zhao1,2, Haifeng Zhao1,3, Zhennan Tian4
1Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu, China.
Abstract:
Tandem light-emitting diodes (LEDs) offer advantages in efficiency, brightness and lower the current density for a target brightness, but their implementation in solution-processed perovskite LEDs is limited by interconnection strategies that introduce high voltage penalties and poor robustness. Here we demonstrate a hierarchically structured interconnection layer (ICL) integrating a near-degenerate charge-generation junction with a crystalline-amorphous oxide composite, enabling low-barrier transport and solvent-tolerant stacking with reduced loss. Using this ICL, we realize double-junction perovskite LEDs in which two subunits operate efficiently in series, achieving a peak external quantum efficiency (EQE) of 42.6%, a maximum radiance of 690 W sr-1 m-2, and low driving voltage. The ICL is compatible with multiple perovskite emitters and supports scalable multijunction integration, yielding multijunction devices with sub-bandgap turn-on voltages and high EQEs exceeding 60%. Our results establish a low-loss interconnection strategy for series-stacked perovskite emitters, providing a practical route toward high-brightness and multi-wavelength perovskite light sources.
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