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Discontinuous Highly Aligned Carbon Fibre Tapes Combined with Bio-Based Polyamide 11
Christian Brauner1, Florian Givel1, Julian Kupski1
1Institute of Polymer Engineering, FHNW University of Applied Sciences and Arts Northwestern Switzerland, Klosterzelgstrasse 2, 5210 Windisch, Switzerland.
This study demonstrates how aligned recycled carbon fibres (rCFs) with bio-based polyamide 11 create sustainable, high-performance composites. Optimized fibre alignment significantly enhances mechanical properties for lightweight applications.
Area of Science:
- Materials Science
- Composite Materials
- Sustainable Engineering
Background:
- Increasing availability of recycled carbon fibres (rCFs) presents opportunities for sustainable composites.
- Discontinuous nature of rCFs necessitates efficient alignment and consolidation techniques.
- Bio-based polymers offer a sustainable alternative to conventional matrix materials.
Purpose of the Study:
- To manufacture highly aligned discontinuous rCF tapes using recycled carbon staple fibres and bio-based polyamide 11 (PA11).
- To investigate the effect of fibre content on the microstructure and mechanical performance of the resulting composites.
- To evaluate the correlation between fibre architecture and mechanical properties.
Main Methods:
- Textile-based processing route for fibre alignment.
- Compression moulding for laminate fabrication.
- Characterization of fibre volume content (FVC), fibre orientation, and mechanical properties (tensile, compression, shear).
- 2D mesoscopic image analysis for fibre orientation distribution.
Main Results:
- Achieved FVC up to 56.72 vol.% for 70 wt.% rCF material.
- Significant increase in tensile stiffness (48.1 GPa) and strength (866 MPa) with higher fibre content.
- Pronounced preferential fibre orientation (69% within ±10°).
- Alignment coefficient (η0) correlated well with tensile modulus, highlighting the importance of fibre architecture.
Conclusions:
- The combination of bio-based PA11 and oriented rCFs offers a promising route to sustainable lightweight composites.
- Textile-based alignment technologies are effective for processing discontinuous rCFs.
- Optimized mesoscopic fibre architecture is crucial for enhancing composite mechanical performance.
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