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Shell filling and exchange coupling in metallic single-walled carbon nanotubes
Wenjie Liang1, Marc Bockrath, Hongkun Park
1Department of Chemistry and Chemical Biology, Harvard University, Cambridge, Massachusetts 02138, USA.
Physical Review Letters
|March 23, 2002
Abstract:
We report the characterization of electronic shell filling in metallic single-walled carbon nanotubes by low-temperature transport measurements. Nanotube quantum dots with average conductance approximately (1-2)e(2)/h exhibit a distinct four-electron periodicity for electron addition as well as signatures of Kondo and inelastic cotunneling. The Hartree-Fock parameters that govern the electronic structure of metallic nanotubes are determined from the analysis of transport data using a shell-filling model that incorporates the nanotube band structure and Coulomb and exchange interactions.