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Updated: Jul 13, 2026

Determination of the Excitation and Coupling Rates Between Light Emitters and Surface Plasmon Polaritons
Published on: July 21, 2018
Theory of molecular excitation and relaxation near a plasmonic device
Gérard Colas des Francs1, Christian Girard, Thierry Laroche
1Institut Carnot de Bourgogne, CNRS UMR5209, Université de Bourgogne, 9 Avenue A. Savary, F-21078 Dijon, France. gerard.colas-des-francs@u-bourgogne.fr
Abstract:
The new optical concepts currently developed in the research field of plasmonics can have significant practical applications for integrated optical device miniaturization as well as for molecular sensing applications. Particularly, these new devices can offer interesting opportunities for optical addressing of quantum systems. In this article, we develop a realistic model able to explore the various functionalities of a plasmon device connected to a single fluorescing molecule. We show that this theoretical method provides a useful framework to understand how quantum and plasmonic entities interact in a small area. Thus, the fluorescence signal evolution from excitation control to relaxation control depending on the incident light power is clearly observed.
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