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Updated: Jun 22, 2026

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Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Pulse compression of submillijoule few-optical-cycle infrared laser pulses using chirped mirrors
Mathieu Giguère1, Bruno E Schmidt, Andrew D Shiner
1Institut National de la Recherche Scientifique, Centre Energie Matériaux et Télécommunications, 1650 Boulevard Lionel-Boulet, Varennes, Quebec J3X1S2, Canada.
Optics Letters
|June 17, 2009
Abstract:
We report generation of 400 microJ, 13.1 fs, 1425 nm optical parametric amplifier laser pulses. Spectral broadening of a 100 Hz optical parametric amplifier laser source is achieved by self-phase modulation in an argon-filled hollow-core fiber, and dispersion compensation is performed using chirped mirrors. This laser source will be useful for ultrafast time-resolved molecular orbital tomography.

