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High Resolution Phonon-assisted Quasi-resonance Fluorescence Spectroscopy
Published on: June 28, 2016
Two-level ultrabright single photon emission from diamond nanocrystals
Igor Aharonovich1, Stefania Castelletto, David A Simpson
1School of Physics, University of Melbourne, Parkville, Victoria 3010, Australia. i.aharonovich@pgrad.unimelb.edu.au
Nano Letters
|August 13, 2009
Summary
Stable, ultrabright single photon sources were created at room temperature using diamond nanocrystals. These sources are ideal for quantum technologies and cellular biomarker applications.
Area of Science:
- Quantum optics
- Materials science
- Nanotechnology
Background:
- Development of stable, room-temperature single photon sources is crucial for quantum technologies.
- Existing sources often suffer from instability or require cryogenic cooling.
- Color centers in diamond offer potential for efficient light emission.
Purpose of the Study:
- To fabricate and characterize stable, ultrabright single photon sources operating at room temperature.
- To evaluate the suitability of these sources for quantum photonics, communication, and cellular biomarking.
Main Methods:
- Fabrication of diamond nanocrystals on a sapphire substrate using chemical vapor deposition (CVD).
- Characterization of the color center's electronic behavior and optical properties.
- Measurement of count rate, emission wavelength, spectral width, and excited state lifetime.
Main Results:
- Achieved stable single photon emission at room temperature.
- Maximum measured count rate of 3.2 x 10^6 counts/s at saturation.
- Emission centered at ~756 nm with a 11 nm FWHM and a 3.7 ns excited state lifetime.
Conclusions:
- The fabricated diamond-based single photon source demonstrates high brightness and stability at room temperature.
- Its properties make it a promising candidate for quantum photonics, secure communication, and advanced cellular imaging.
- This work advances the development of practical quantum technologies and bio-imaging tools.
