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Related Experiment Video

Updated: Jun 20, 2026

Hyperpolarized Xenon for NMR and MRI Applications
16:20

Hyperpolarized Xenon for NMR and MRI Applications

Published on: September 6, 2012

Two-photon resonant upconversion in xenon.

Y M Yiu, K D Bonin, T J McIlrath

    Optics Letters
    |August 28, 2009
    PubMed
    Summary
    This summary is machine-generated.

    Researchers generated coherent vacuum ultraviolet (VUV) radiation using xenon gas and two-photon resonances. This method achieved high-efficiency VUV light generation for various applications.

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    Published on: October 23, 2018

    Area of Science:

    • Atomic, Molecular, and Optical Physics
    • Nonlinear Optics
    • Quantum Electronics

    Background:

    • Generation of coherent vacuum ultraviolet (VUV) radiation is crucial for various spectroscopic and materials science applications.
    • Four-wave mixing (FWM) is a nonlinear optical process used to generate new frequencies, but efficiency can be limited.
    • Two-photon resonances can significantly enhance nonlinear optical processes by increasing the interaction probability.

    Purpose of the Study:

    • To investigate the generation of coherent VUV radiation using four-wave mixing enhanced by two-photon resonances in xenon.
    • To determine the optimal conditions (e.g., xenon pressure) for maximizing VUV generation efficiency and output intensity.
    • To explore the potential for parametric generation at specific VUV wavelengths.

    Main Methods:

    • Employed four-wave mixing (FWM) processes in xenon gas.
    • Utilized two-photon resonances to enhance the nonlinear interaction.
    • Varied xenon pressure to optimize phase-matching conditions and observed output intensities at specific VUV wavelengths (e.g., 125.9, 126.1, 125.4 nm).

    Main Results:

    • Successfully generated coherent VUV radiation at wavelengths including 125.9, 126.1, and 125.4 nm.
    • Achieved maximum conversion efficiencies on the order of 10⁻⁴.
    • Observed maximum output intensities for difference frequency generation (2ω₁ - ω₂) at specific xenon pressures and phase mismatch values for different resonant states (7p[0 (1/2)](0), 7p[1 (1/2)](2), and 6p' [1 (1/2)](2)). Parametric generation at 117.0 nm via the 7s[1(1/2)](0)(1) state was also noted.

    Conclusions:

    • Two-photon resonances significantly enhance four-wave mixing processes in xenon for VUV generation.
    • Optimizing xenon pressure is critical for achieving efficient VUV generation by controlling phase-matching conditions.
    • The demonstrated method provides a viable route for generating tunable coherent VUV radiation.