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Updated: Mar 28, 2026

Elemental-sensitive Detection of the Chemistry in Batteries through Soft X-ray Absorption Spectroscopy and Resonant Inelastic X-ray Scattering
Published on: April 17, 2018
The LCLS variable-energy hard X-ray single-shot spectrometer.
David Rich1, Diling Zhu1, James Turner1
1Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA.
A new hard X-ray single-shot spectrometer (HXSSS) enables precise measurement of the LCLS free-electron laser (FEL) spectrum. This advancement aids experimental users and accelerator physicists in optimizing FEL performance.
Area of Science:
- X-ray spectroscopy
- Accelerator physics
- Free-electron laser technology
Background:
- Accurate characterization of free-electron laser (FEL) spectra is crucial for experimental success and accelerator optimization.
- Existing methods may lack the necessary resolution or single-shot capability for dynamic FEL processes.
- The Linac Coherent Light Source (LCLS) requires advanced diagnostics for its high-intensity X-ray beams.
Purpose of the Study:
- To report the design, implementation, and performance of a novel variable-energy hard X-ray single-shot spectrometer (HXSSS).
- To provide single-shot spectral measurements for LCLS FEL users and accelerator physicists.
- To validate the HXSSS's capability for optimizing FEL performance and lasing mechanisms.
Main Methods:
- Utilized a cylindrically bent silicon thin crystal for polychromatic X-ray beam dispersion.
- Employed a detector system comprising a Ce:YAG scintillator, optical imaging, and a low-noise pixelated camera.
- Integrated the spectrometer into the LCLS experimental environment for real-time spectral analysis.
Main Results:
- Achieved single-shot spectrum measurements with a spectral range exceeding 2% and a resolution of 2 × 10⁻⁵.
- Successfully operated within the designed energy range of 4 to 20 keV.
- Demonstrated the HXSSS's effectiveness during commissioning, meeting all performance goals.
Conclusions:
- The HXSSS is a high-performance instrument for characterizing hard X-ray FEL spectra.
- It significantly enhances the capabilities for FEL research and accelerator development at LCLS.
- The spectrometer's single-shot capability is vital for experiments sensitive to FEL spectral variations.
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