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Imaging Plasmonic Fields with Atomic Spatiotemporal Resolution.

Jianxiong Li1, Erfan Saydanzad1, Uwe Thumm1

  • 1Department of Physics, Kansas State University, Manhattan, Kansas 66506, USA.

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|June 16, 2018
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Summary
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We present a new method to reconstruct plasmonic near fields at nanoparticles using infrared-streaked extreme-ultraviolet photoemission spectroscopy. This technique achieves subfemtosecond temporal and subnanometer spatial resolution for imaging transient plasmonic fields.

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Area of Science:

  • Plasmonics
  • Nanophotonics
  • Ultrafast Spectroscopy

Background:

  • Plasmonic near fields are crucial for nanoscale light manipulation.
  • Characterizing transient plasmonic fields with high spatiotemporal resolution is challenging.

Purpose of the Study:

  • To develop a novel scheme for reconstructing plasmonic near fields.
  • To demonstrate high-resolution imaging of transient plasmonic fields at nanoparticle surfaces.

Main Methods:

  • Utilizing infrared-streaked extreme-ultraviolet photoemission spectra.
  • Employing quantum-mechanically modeled spectra for analysis.
  • Simulating plasmonic fields at gold nanospheres and nanoshells.

Main Results:

  • Accurate reconstruction of transient plasmonic fields demonstrated.
  • Achieved subfemtosecond temporal resolution.
  • Achieved subnanometer spatial resolution.

Conclusions:

  • The proposed scheme enables precise imaging of dynamic plasmonic phenomena.
  • This method offers unprecedented resolution for studying light-matter interactions at the nanoscale.