UV-SWIR broad range photodetectors made from few-layer α-In₂Se₃ nanosheets

Photodetectors are very important for many applications. However, inexpensive infrared photodetectors with high performance at room temperature are still rare. Furthermore, it is still a great challenge to realize on-chip wide-spectrum detection by using conventional photodetectors. van der Waals semiconductors are promising for high performance optoelectronic devices. Here, we report broad range photodetectors made from few-layer α-In2Se3 nanosheets. The photodetectors show response in an unexpected broad range from ultraviolet (325 nm) to short-wavelength infrared (1800 nm) at room temperature. The optical response in the long wavelengths beyond the bandgap is attributed to oxygen absorption and oxygen-associated selenium defects in In2Se3, supported by theoretical simulation and controlled experiments. High responses to 700 nm and 1550 nm lasers are demonstrated on the same In2Se3 device. The stability of In2Se3 under the atmosphere at room temperature and the low power consumption of the devices make the In2Se3 photodetectors promising for optoelectronic applications.