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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Polymerized Ionic Liquid-Containing Interpenetrating Network Solid Polymer Electrolytes for All-Solid-State Lithium

Xiaowei Li1, Yongwei Zheng1, Qiwei Pan1

  • 1Department of Materials Science and Engineering , Drexel University , Philadelphia , Pennsylvania 19104 , United States.

ACS Applied Materials & Interfaces
|September 3, 2019
PubMed
Summary
This summary is machine-generated.

This study introduces a new solid polymer electrolyte (SPE) for lithium metal batteries (LMBs). The novel material enhances ionic conductivity and lithium dendrite resistance, improving battery performance and stability.

Keywords:
hybrid electrolyteslithium metal batteriespolyhedral oligomeric silsesquioxanes (POSS)polymerized ionic liquidsolid polymer electrolytes

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Polymer Chemistry

Background:

  • Lithium metal batteries (LMBs) offer high energy density but suffer from uneven lithium deposition.
  • This uneven deposition leads to dendrite formation, hindering practical application and safety.
  • Developing stable solid polymer electrolytes (SPEs) is crucial for overcoming these limitations.

Purpose of the Study:

  • To develop a novel interpenetrating polymer network solid polymer electrolyte (IPN SPE) for stabilizing lithium electrodeposition in LMBs.
  • To improve the ionic conductivity and lithium dendrite resistance of SPEs.
  • To enhance the overall battery performance and cycle life of LMBs.

Main Methods:

  • Synthesized an IPN SPE by incorporating a polymerized ionic liquid (PIL), poly(diallyldimethylammonium) bis(trifluoromethanesulfonyl)imide, into a polyhedral oligomeric silsesquioxane-poly(ethylene glycol)-based network.
  • Characterized the IPN SPE's ionic conductivity, lithium dendrite resistance, and electrochemical stability.
  • Conducted galvanostatic cycling and polarization measurements to analyze ion transport and distribution.
  • Performed full battery tests to evaluate discharge capacity, cycle life, and Coulombic efficiency.

Main Results:

  • The novel IPN SPE demonstrated significantly improved ionic conductivity compared to the virgin SPE.
  • The IPN SPE exhibited excellent resistance to lithium dendrite formation.
  • Homogeneous ion distribution and an immobilized ion network were observed in the PIL-containing IPN SPE.
  • Full battery tests confirmed superior discharge capacity, extended cycle life, and high Coulombic efficiency.

Conclusions:

  • The developed PIL-containing IPN SPE effectively stabilizes lithium electrodeposition.
  • This novel material presents a promising strategy for fabricating high-performance and safe lithium metal batteries.
  • The findings highlight the potential of IPN SPEs in advancing next-generation energy storage solutions.