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Updated: Dec 17, 2025

Core/shell Printing Scaffolds For Tissue Engineering Of Tubular Structures
05:52

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Published on: September 27, 2019

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Lignin-Based Direct Ink Printed Structural Scaffolds.

Bo Jiang1, Yonggang Yao1, Zhiqiang Liang1

  • 1Department of Materials Science and Engineering, University of Maryland, College Park, MD, 20742, USA.

Small (Weinheim an Der Bergstrasse, Germany)
|June 30, 2020
PubMed
Summary
This summary is machine-generated.

Researchers developed a 3D printing method for lignin, a sustainable biomass component. This lignin-based ink creates robust, water-stable structures, outperforming traditional cellulose-based 3D prints.

Keywords:
3D printinginkligninstructural scaffoldswood inspired

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Area of Science:

  • Biomaterials Engineering
  • Sustainable Materials
  • Additive Manufacturing

Background:

  • Lignocellulosic biomass is an abundant, sustainable resource for 3D printing applications.
  • Cellulose-based 3D prints are fragile and water-intolerant due to their hydrophilic nature and porous structure.
  • Lignin, a key component of lignocellulose, has not been utilized for 3D printing due to poor rheological properties.

Purpose of the Study:

  • To develop a direct ink writing strategy for fabricating 3D structures using unrefined lignin.
  • To overcome the rheological challenges associated with lignin for 3D printing applications.
  • To create lignin-based 3D structures with enhanced mechanical properties, stability, and functionality compared to cellulose.

Main Methods:

  • A low-cost direct ink printing strategy was employed using unrefined lignin.
  • A soft triblock copolymer was utilized as a crosslinking agent to tailor ink rheology.
  • Lignin-based inks were characterized for rheological behavior, water content, microstructure, and mechanical strength.

Main Results:

  • Lignin-based inks exhibited adjustable rheology, enabling soft to rigid structures and vertical printing.
  • Printed lignin structures showed a denser microstructure with significantly higher wet tensile strength (≈30 MPa) compared to cellulose (≈0.6 MPa).
  • Lignin-based materials demonstrated improved stability in water and under heat, along with UV-blocking capabilities.

Conclusions:

  • A novel, low-cost 3D printing method for unrefined lignin was successfully developed.
  • Lignin-based 3D printed materials offer superior mechanical strength, stability, and functionality over cellulose.
  • This advancement opens new avenues for utilizing lignin in sustainable and high-performance 3D printed applications.