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Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes.

Abhik Banerjee1,2, Xuefeng Wang1,3, Chengcheng Fang1

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Interfaces in all-solid-state batteries (ASSBs) limit performance. Understanding and engineering these solid-solid interfaces is key to developing safer, high-energy ASSBs for future applications.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) are crucial for safe, high-energy storage.
  • High interfacial resistance, not ion diffusion, limits ASSB performance.
  • Diverse interfaces (physical, grain boundaries, chemical reactions) increase resistance.

Purpose of the Study:

  • To review distinctive features of ASSB interfaces and interphases.
  • To summarize recent work on identifying, probing, understanding, and engineering these interfaces.
  • To highlight the importance of interphase properties for stable interface design.

Main Methods:

  • Review of existing literature on ASSB interfaces.
  • Analysis of interphase characteristics (composition, distribution, electronic/ionic properties).
  • Discussion of characterization methods for dynamic and buried interfaces.

Main Results:

  • Interfacial resistance significantly impacts ASSB Coulombic efficiency, power, and lifespan.
  • Understanding cathode-electrolyte and electrolyte-anode interphase properties is critical.
  • Mechanical behavior of interfaces and ASSB components is vital, especially with Li metal anodes.

Conclusions:

  • Engineering stable interfaces is essential for practical, high-energy ASSBs.
  • Comprehensive characterization methods are needed to understand complex interfaces.
  • Addressing interfacial challenges is key to unlocking ASSB potential.