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A battery is a galvanic cell that is used as a source of electrical power for specific applications. Modern batteries exist in a multitude of forms to accommodate various applications, from tiny button batteries such as those that power wristwatches to the very large batteries used to supply backup energy to municipal power grids. Some batteries are designed for single-use applications and cannot be recharged (primary cells), while others are based on conveniently reversible cell reactions that...
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Few compounds act as strong acids. A far greater number of compounds behave as weak acids and only partially react with water, leaving a large majority of dissolved molecules in their original form and generating a relatively small amount of hydronium ions. Weak acids are commonly encountered in nature, being the substances partly responsible for the tangy taste of citrus fruits, the stinging sensation of insect bites, and the unpleasant smells associated with body odor. A familiar example of a...
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Ionic crystals consist of two or more different kinds of ions that usually have different sizes. The packing of these ions into a crystal structure is more complex than the packing of metal atoms that are the same size.
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In a galvanic cell, the electrical work is done by a redox system on its surroundings as electrons produced by the spontaneous redox reactions are transferred through an external circuit. Alternatively, an external circuit does work on a redox system by imposing a voltage sufficient to drive an otherwise nonspontaneous reaction in a process known as electrolysis. For instance, recharging a battery involves the use of an external power source to drive the spontaneous (discharge) cell reaction in...
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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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Lithium/Sulfide All-Solid-State Batteries using Sulfide Electrolytes.

Jinghua Wu1,2, Sufu Liu3, Fudong Han3

  • 1Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang, 315201, P. R. China.

Advanced Materials (Deerfield Beach, Fla.)
|August 20, 2020
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Summary
This summary is machine-generated.

All-solid-state lithium batteries (ASSLBs) utilize sulfide electrolytes for high conductivity and safety. Challenges like stability and dendrite formation are addressed for next-generation energy storage.

Keywords:
all-solid-state lithium batterieslithium-sulfur batteriessulfide cathodessulfide electrolytes

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state lithium batteries (ASSLBs) offer enhanced safety and energy density over conventional batteries.
  • Solid-state electrolytes are crucial for ASSLB performance, with sulfide electrolytes showing high ionic conductivity.

Purpose of the Study:

  • To review emerging sulfide electrolytes and their preparation methods for ASSLBs.
  • To highlight critical properties of sulfide electrolytes, including electrochemical stability and electrode interface compatibility.
  • To discuss opportunities for advancing sulfide-based ASSLBs.

Main Methods:

  • Literature review of sulfide electrolytes and preparation techniques.
  • Analysis of required properties for sulfide electrolytes in ASSLBs.
  • Discussion of challenges and future prospects.

Main Results:

  • Sulfide electrolytes exhibit ionic conductivity comparable to or exceeding liquid electrolytes.
  • Key challenges include narrow electrochemical stability windows and unstable electrode interfaces.
  • Lithium dendrite formation remains a significant concern.

Conclusions:

  • Sulfide electrolytes are promising for ASSLBs due to high ionic conductivity and interface compatibility.
  • Addressing stability and interface issues is crucial for practical application.
  • Further research into preparation methods and property optimization is needed.