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Updated: Nov 5, 2025

12:21
Stimulated Stokes and Antistokes Raman Scattering in Microspherical Whispering Gallery Mode Resonators
Published on: April 4, 2016
11.4K
Fine structure of second-harmonic resonances in χ(2) optical microresonators
Optics Express
|May 14, 2021
Summary
This study models second-harmonic generation in whispering gallery resonators (WGRs) with frequency detunings. The model accurately predicts resonance distortions and efficiency, validated by lithium niobate WGR experiments.
Area of Science:
- Nonlinear optics
- Photonics
- Resonator physics
Background:
- Whispering gallery resonators (WGRs) offer unique optical properties but face challenges in simultaneous resonance and phase-matching for nonlinear processes like second-harmonic generation (SHG).
- Discrete frequency spectra of WGRs often prevent simultaneous fulfillment of resonance and phase-matching conditions for interacting waves.
Purpose of the Study:
- To develop a theoretical model for second-harmonic generation (SHG) in whispering gallery resonators (WGRs) that accounts for non-zero frequency detunings.
- To investigate the impact of frequency detunings on resonance line shapes and SHG efficiency in WGRs.
- To experimentally validate the developed model using a lithium niobate WGR.
Main Methods:
- Development of a theoretical model for SHG in WGRs incorporating pump and second-harmonic frequency detunings.
- Analysis of resonance line shape distortions based on relative linewidths.
- Experimental implementation using a lithium niobate WGR to measure SHG efficiency as a function of detuning.
- Comparison of experimental results with model predictions for both lithium niobate and cadmium silicon phosphide WGRs.
Main Results:
- The model predicts significant distortions in pump and second-harmonic resonance line shapes when linewidths are similar, which are absent when the second-harmonic linewidth is much larger.
- The SHG efficiency is accurately described as a function of detuning.
- Excellent quantitative agreement was achieved between the model predictions and experimental results for SHG efficiency in a lithium niobate WGR.
- The model correctly predicted the absence of resonance distortions in the lithium niobate WGR and their presence in the cadmium silicon phosphide WGR, correlating with their respective resonance linewidths.
Conclusions:
- The developed model provides an accurate description of second-harmonic generation in whispering gallery resonators with frequency detunings.
- The study highlights the crucial role of resonance linewidths in determining the line shape distortions and overall SHG performance.
- Experimental validation confirms the model's predictive power for optimizing nonlinear optical processes in WGRs.
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