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Coherent Surface Plasmon Hole Burning via Spontaneously Generated Coherence.

Habibur Rahman1, Hazrat Ali2, Rafi Ud Din3

  • 1Department of Physics, University of Malakand Chakdara Dir Lower, Malakand 23050, Pakistan.

Molecules (Basel, Switzerland)
|November 13, 2021
PubMed
Summary

This study theoretically investigates surface plasmon (SP)-induced spectral hole burning (SHB). Introducing spontaneous generated coherence (SGC) enhances SHB and enables slow surface plasmon polariton (SPP) propagation for advanced applications.

Keywords:
plasmon hole burningsilver mediumspontaneously generated coherence

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Area of Science:

  • Photonics
  • Plasmonics
  • Quantum Optics

Background:

  • Surface plasmon (SP) phenomena are crucial for light-matter interactions at interfaces.
  • Spectral hole burning (SHB) is a technique used to study optical properties of materials.
  • Surface plasmon polaritons (SPPs) are electromagnetic waves propagating at metal-dielectric interfaces.

Purpose of the Study:

  • To theoretically investigate SP-induced SHB at the silver-dielectric interface.
  • To explore the effect of spontaneous generated coherence (SGC) on SHB and SPP propagation.
  • To demonstrate enhanced SPP propagation length for potential applications.

Main Methods:

  • Theoretical investigation of SP-induced SHB.
  • Modeling the influence of spontaneous generated coherence (SGC) on SPP dispersion and absorption.
  • Analyzing the spectral hole burning dip and SPP propagation length.

Main Results:

  • Observed a lamb dip in the absorption spectrum of SPPs, reducing absorption at selective frequencies.
  • Demonstrated that SGC normalizes dispersion slope and enables slow SPP propagation.
  • Showcased enhanced SHB dip and significantly increased SPP propagation length (up to 600 µm) under SGC.

Conclusions:

  • SGC significantly enhances plasmon hole burning.
  • Controlled modification of SHB is achievable via driving fields.
  • Enhanced plasmon hole burning and slow SPP propagation offer promising applications in sensing, optical communication, and nano-photonics.