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Carrier-mediated ferromagnetism in two-dimensional PtS2
Konstantina Iordanidou1, Michel Houssa2, Clas Persson1
1Centre for Materials Science and Nanotechnology, Department of Physics, University of Oslo P.O. Box 1048 Blindern NO-0316 Oslo Norway konstantina.iordanidou@smn.uio.no.
Abstract:
Using first principles calculations based on density functional theory, we study the impact of hole doping on the magnetic and electronic properties of two dimensional PtS2. Although 2D PtS2 is intrinsically non-magnetic, a stable ferromagnetic phase is found for a wide range of hole densities, owing to the so-called Stoner instabilities. Besides spontaneous magnetization, half-metallicity is additionally observed. The majority and minority spin states exhibit insulating and metallic nature, respectively, allowing a fully polarized spin transport in 2D PtS2. Lastly, hole doping resulting from substitutional doping is investigated. For As-doped PtS2 shallow spin-polarized states close to the valence band edge are observed, and among all studied group-V dopants, As replacing S, is the most promising one to induce p-type conductivity and a subsequent ferromagnetic order in PtS2.
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