Improved Bounds on Ultralight Scalar Dark Matter in the Radio-Frequency Range

We present a search for fundamental constant oscillations in the range 20 kHz-100 MHz that may arise within models for ultralight dark matter (UDM). Using two independent optical-spectroscopy apparatuses, we achieve up to ×1000 greater sensitivity in the search relative to previous work [D. Antypas et al., Phys. Rev. Lett. 123, 141102 (2019).PRLTAO0031-900710.1103/PhysRevLett.123.141102]. We report no observation of UDM and thus constrain respective couplings to electrons and photons within the investigated UDM particle mass range 8×10^{-11}-4×10^{-7}  eV. The constraints significantly exceed previously set bounds from atomic spectroscopy and, as we show, may surpass in future experiments those provided by equivalence-principle (EP) experiments in a specific case regarding the combination of UDM couplings probed by the EP experiments.