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Biomimetic control of charge transfer in MOFs by solvent coordination for boosting photocatalysis
Zejin Wang1,2, Rui Ding3, Jie Zhang1,2
1School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210033, P. R. China. wangy@nju.edu.cn.
Chemical Communications (Cambridge, England)
|August 17, 2022
Abstract:
The role of the coordination solvent in MOFs with photocatalysis can't be ignored. Novel [Ni(PTCA)·sol]-MOFs with a 3D open wavy-layered structure are selected for in-depth study by imitating the internal environment of a chameleon. The results confirm that the coordination solvent can modulate the band structure and the polarity is the key to accelerate the formation of intermediate H*.
