Quantum Dot-based Luminescent Solar Concentrators Fabricated through the Ultrasonic Spray-Coating Method
Junyu Wang1, Yucheng Yuan1, Jeremy Schneider1
1Department of Chemistry, Brown University, Providence, Rhode Island 02912, United States.
ACS Applied Materials & Interfaces
|August 31, 2022
Summary
Researchers developed a new ultrasonic spray method for fabricating high-performance quantum dot (QD)-based luminescent solar concentrators (LSCs). This scalable technique enables precise control over QD-LSC dimensions and performance for building-integrated photovoltaics.
Area of Science:
- Materials Science
- Renewable Energy Engineering
- Nanotechnology
Background:
- Luminescent solar concentrators (LSCs) are wave-guiding devices for concentrating solar light onto photovoltaic cells.
- LSCs integrated with photovoltaic devices (PVs) offer potential for net-zero-energy buildings, particularly in facade applications.
- Scalable, adaptable, and controllable fabrication methods for LSCs are crucial for their practical implementation.
Purpose of the Study:
- To introduce and evaluate an ultrasonic nebulization-assisted spray deposition technique for fabricating quantum dot-based LSCs (QD-LSCs).
- To demonstrate the capability of this method for producing high-performance QD-LSCs with customizable dimensions and geometries.
- To highlight the method's robustness in controlling thin-film quality, independent of ink concentration and volume, for performance optimization.
Main Methods:
- Fabrication of QD-LSCs using an ultrasonic nebulization-assisted spray deposition technique.
- Utilizing quantum dots (QDs) as the luminescent material within the LSC devices.
- Characterization of QD-LSC performance and thin-film properties.
Main Results:
- Successful fabrication of high-performance QD-LSCs with varying device dimensions and geometries.
- Demonstrated independence of QD thin-film coating quality from ink concentration and volume.
- Enabled precise programming and optimization of QD-LSC device performance.
Conclusions:
- The ultrasonic spray coating method is a reliable and scalable technique for manufacturing high-quality QD-LSCs.
- This method facilitates the integration of QD-LSCs into diverse applications, including building facades.
- The developed technique supports the advancement of LSC technology for efficient solar energy harvesting.


