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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Rational Optimization of Cathode Composites for Sulfide-Based All-Solid-State Batteries.

Artur Tron1, Raad Hamid1, Ningxin Zhang1

  • 1AIT Austrian Institute of Technology GmbH, Center for Low-Emission Transport, Battery Technologies, Giefinggasse 2, 1210 Vienna, Austria.

Nanomaterials (Basel, Switzerland)
|January 21, 2023
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Summary
This summary is machine-generated.

Optimizing composite cathodes is crucial for high-performance all-solid-state lithium-ion batteries. This study systematically investigates key formulation parameters for improved cycling stability and battery performance.

Keywords:
Li6PS5Clall-solid-state batteryargyroditelithium batteryprocessing

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state lithium-ion batteries (ASSLIBs) utilize solid electrolytes for enhanced safety and energy density.
  • Argyrodite solid electrolytes offer high ionic conductivity, but cathode formulation remains a performance bottleneck.
  • Current research often lacks comprehensive analysis of electrode parameters, hindering direct comparison.

Purpose of the Study:

  • To systematically investigate and optimize key parameters in composite cathode preparation for ASSLIBs.
  • To elucidate the influence of various formulation factors on the electrochemical cycling performance.
  • To provide a rational approach for designing high-performance composite cathodes.

Main Methods:

  • Investigation of powder electrodes without binders to optimize active material morphology, conductive additive, solid electrolyte particle size, and active material-to-electrolyte ratio.
  • Examination of cast electrodes to assess the impact of binder incorporation on cycling performance.
  • Utilizing a rational optimization approach for composite cathodes with solid sulfide electrolytes.

Main Results:

  • Identified critical parameters influencing the cycling performance of composite cathodes.
  • Demonstrated the significant impact of particle morphology, conductive additive, electrolyte particle size, and component ratios.
  • Revealed the role of binders in the electrochemical performance of cast electrodes.

Conclusions:

  • Composite cathode formulation is a critical factor for achieving high performance in ASSLIBs, even with highly conductive solid electrolytes.
  • A systematic, rational approach is essential for optimizing electrode design and overcoming performance limitations.
  • Further research into binder effects is necessary for advanced electrode architectures.