Structural and Scintillation Properties of Ce³⁺:Gd₃Al₃Ga₂O₁₂ Translucent Ceramics Prepared by One-Step Sintering

Cerium-doped gadolinium aluminum gallium garnet (Ce³⁺:Gd₃Al₃Ga₂O₁₂, Ce³⁺:GAGG) ceramic is a promising scintillation material. In this study, Ce³⁺:Gd₃Al₃Ga₂O₁₂ scintillation ceramics were prepared by the one-step sintering of commercially available Gd₂O₃, Al₂O₃, Ga₂O₃, and CeO₂ powders in a flowing oxygen atmosphere at 1600 °C by solid-phase reaction sintering. For all the Ce³⁺:Gd₃Al₃Ga₂O₁₂ ceramic samples doped with different amounts of Ce³⁺ doping, dense ceramics were obtained. The structure, photoluminescence, and scintillation properties of the Ce³⁺:Gd₃Al₃Ga₂O₁₂ ceramics have been investigated. The average grain size of samples sintered at 1600 °C is about 2 μm. The X-ray excitation luminescence peak is around 560 nm, which is consistent with that of Ce³⁺:Gd₃Al₃Ga₂O₁₂ single crystals, matching well with the computed tomography X-ray detector's response sensitivity. The light yield is higher compared to the standard reference sample-lutetium yttrium orthosilicate single crystal.