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Pulsewidth-switchable ultrafast source at 114 nm.

Anahita Omoumi, Michele Natile, Evangelos Papalazarou

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    |September 1, 2023
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    Summary
    This summary is machine-generated.

    We developed a vacuum ultraviolet (VUV) laser source for studying electronic dynamics in solids. This high-repetition-rate VUV source enables advanced time-resolved and angle-resolved photoemission spectroscopy (ARPES) experiments.

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    Area of Science:

    • Ultrafast laser science
    • Solid-state physics
    • Spectroscopy

    Background:

    • Femtosecond laser sources in ultraviolet (UV) and vacuum UV (VUV) are crucial for time-resolved and angle-resolved photoemission spectroscopy (ARPES) in solids.
    • Existing VUV sources often lack the high repetition rates and photon flux required for comprehensive electronic structure studies.

    Purpose of the Study:

    • To develop a compact, high-repetition-rate VUV laser source at 114 nm (10.8 eV).
    • To enable advanced ARPES studies of electronic dynamics across the entire Brillouin zone in various materials.

    Main Methods:

    • Utilized an industrial ytterbium-doped ultrafast laser.
    • Employed nonlinear pulse width selection and two cascaded frequency tripling stages (crystal and xenon gas).
    • Analyzed ionization effects in gas-based third harmonic generation phase-matching through theory, simulations, and experiments.

    Main Results:

    • Successfully generated a VUV source at 114 nm with high photon flux and high repetition rate.
    • Demonstrated adjustable time resolutions for the VUV pulses.
    • Validated the theoretical understanding of ionization's role in phase-matching.

    Conclusions:

    • The developed VUV source is a powerful tool for tabletop ARPES.
    • It facilitates detailed investigations into the electronic dynamics of a wide range of solid materials.
    • The source's capabilities advance the study of electronic band structures and dynamics.