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Polyhedral oligomeric silsesquioxanes (POSS) enhance cesium-halide perovskite structures, improving crystallization and properties. This review explores POSS-perovskite hybrids for advanced materials.

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Area of Science:

  • Materials Chemistry
  • Nanoscale Science

Background:

  • Polyhedral oligomeric silsesquioxanes (POSS) and hybrid organo-halide perovskites are key nanoscale frameworks.
  • Both materials are under intensive investigation for diverse applications.

Purpose of the Study:

  • To review the role of POSS in engineering inorganic cesium-halide perovskites (CsPbX3).
  • To highlight the creation of novel hybrid POSS-perovskite derivatives with enhanced properties.

Main Methods:

  • Literature review focusing on structural specificity and properties of hybrid POSS perovskites.
  • Analysis of POSS as a passivating and structure-controlling agent for perovskites.

Main Results:

  • POSS integration effectively controls perovskite crystallization.
  • Surface defect passivation and engineering of energy/optoelectronic properties are achieved.
  • New hybrid POSS-perovskite materials exhibit improved characteristics.

Conclusions:

  • Combining POSS with cesium-halide perovskites offers a promising strategy for materials development.
  • POSS-perovskite hybrids represent a new class of advanced materials with tunable properties.