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Three-dimensional (3D) moment imaging with a USB3 oscilloscope.

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A new portable USB3 oscilloscope implementation enhances 3D momentum imaging. This technique achieves ~60 picosecond time resolution for broader accessibility in chemical physics research.

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Area of Science:

  • Chemical Physics
  • Spectroscopy
  • Molecular Imaging

Background:

  • 3D momentum imaging is a powerful technique for analyzing molecular dynamics.
  • Previous implementations relied on high-speed digitizers, limiting portability and accessibility.

Purpose of the Study:

  • To report a new, portable implementation of a 3D momentum imaging technique.
  • To replace high-speed digitizers with a USB3 oscilloscope for enhanced accessibility.

Main Methods:

  • A portable USB3 oscilloscope replaced the high-speed digitizer.
  • A novel triggering scheme was developed to minimize jitter and synchronize signals.
  • Performance was validated using laser desorption/ionization of 2,5-dihydroxybenzoic acid.

Main Results:

  • Achieved a time resolution of approximately 60 picoseconds for time-of-flight measurements.
  • Maintained a count rate of approximately 1 kHz, comparable to previous systems.
  • Demonstrated the portability and accessibility of the upgraded 3D momentum imaging setup.

Conclusions:

  • The new implementation offers comparable performance to existing systems with significantly improved portability.
  • This advancement makes high-performing 3D momentum imaging more accessible to researchers.
  • The portable setup facilitates wider application in chemical physics and related fields.