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Area of Science:

  • Materials Science
  • Electrochemistry
  • Battery Technology

Background:

  • Sulfide solid-state batteries offer high ionic conductivity and good mechanical properties.
  • Complex solid-solid interfaces hinder fast rate and long cycling performance in these batteries.

Purpose of the Study:

  • To comprehensively assess factors determining cell performance in sulfide-based solid-state batteries.
  • To disentangle interfacial processes affecting battery components: high-voltage cathode, sulfide separator, and lithium metal anode.

Main Methods:

  • Utilized a multiconfigurational approach.
  • Applied advanced deconvolution of electrochemical impedance signals using distribution of relaxation times.

Main Results:

  • Identified multiple impedance sources from cathode, separator, and anode interfaces.
  • Found cycling performance is sensitive to cathode chemomechanics, SEI formation, and Li diffusion.

Conclusions:

  • Interfacial processes significantly impact overall performance of lithium metal solid-state batteries.
  • Results aid in designing improved sulfide solid-state batteries and assessing battery aging.